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- W2595588520 abstract "We have studied the elasticity of low volume fraction hyaluronic acid polyelectrolyte gels in swelling equilibrium as a function of salt concentration and strand length. By measuring the shear modulus at different salt concentrations for a constant volume fraction, and for different volume fractions at constant salt concentrations, we uniquely identify the physical parameters responsible for swelling, the chain hydrophobicity, χ, and the degree of ionization of the network, α, for our experimental conditions. Using these parameters, we predict the complex relationship between the elasticity of the network and the polymer volume fraction. The relationship is nonmonotonic due to the internal pressure of the system, and we predict that even in the equilibrium linear-elastic regime, polyelectrolyte gels stiffen as they swell in low salt solutions. For higher salt concentrations, the relationship is reversed, and the modulus increases with polymer volume fraction as expected. Using dynamic light scattering and..." @default.
- W2595588520 created "2017-03-23" @default.
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- W2595588520 date "2017-03-17" @default.
- W2595588520 modified "2023-09-29" @default.
- W2595588520 title "Elasticity at Swelling Equilibrium of Ultrasoft Polyelectrolyte Gels: Comparisons of Theory and Experiments" @default.
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- W2595588520 doi "https://doi.org/10.1021/acs.macromol.6b02656" @default.
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