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• W2597651109 endingPage "5034" @default.
• W2597651109 startingPage "5031" @default.
• W2597651109 abstract "A new reactivity pattern of Rh2(II)-N-arylnitrenes was discovered that facilitates the synthesis of medium-sized N-heterocycles from ortho-cyclobutanol-substituted aryl azides. The key ring-expansion step of the catalytic cycle is both chemoselective and stereospecific. Our mechanistic experiments implicate the formation of a rhodium N-arylnitrene catalytic intermediate and reveal that sp3 C–H bond amination of this electrophilic species is competitive with the ring-expansion process." @default.
• W2597651109 created "2017-04-07" @default.
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• W2597651109 creator A5089663290 @default.
• W2597651109 date "2017-03-29" @default.
• W2597651109 modified "2023-10-16" @default.
• W2597651109 title "Rh₂(II)-Catalyzed Ring Expansion of Cyclobutanol-Substituted Aryl Azides To Access Medium-Sized <i>N</i>-Heterocycles" @default.
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• W2597651109 doi "https://doi.org/10.1021/jacs.7b01833" @default.
• W2597651109 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/28355068" @default.
• W2597651109 hasPublicationYear "2017" @default.
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