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• W2598985850 abstract "Triarylamines oxidized to radical cations can be used as stable spins sources for the design of high-spin compounds. Here, we present the synthesis of the polyarylamine-containing hexaazacyclophanes linked via meta-terphenyl bridges. Spins, created after oxidation of the polymer, can be coupled magnetically in cyclophane moieties via meta-phenyl and along the polymer chain via meta-terphenyl units. The formation of a quintet spin state was evidenced by pulsed-EPR nutation spectroscopy. Two exchange coupling constants via both couplers were determined experimentally and corresponded to J/k = 89 K in the cyclophane moiety and j/k = 17 K via meta-terphenyl. Most importantly, in this polymer, four spins can be ferromagnetically ordered via both couplers, which leads to the high spin state." @default.
• W2598985850 created "2017-04-07" @default.
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• W2598985850 date "2017-04-07" @default.
• W2598985850 modified "2023-10-11" @default.
• W2598985850 title "High-Spin Polymers: Ferromagnetic Coupling of <i>S</i> = 1 Hexaazacyclophane Units up to a Pure <i>S</i> = 2 Polycyclophane" @default.
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• W2598985850 doi "https://doi.org/10.1021/acs.jpcb.7b01531" @default.
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