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- W2599523653 abstract "Abstract Since the first demonstration by Fujishima and Honda of photoelectrochemical water splitting, this route to renewable hydrogen fuel has been pursued with great endeavor. The oxidation of water has been identified as the kinetic “bottleneck” limiting the overall reaction efficiency, thus there is a pressing need to develop more active photocatalysts that can drive this reaction. Some of the most promising materials that can oxidize water are metal oxide semiconductors. The most popular metal oxide photoanodes for water oxidation are TiO 2 , α-Fe 2 O 3 , BiVO 4, and WO 3 , but even state-of-the-art examples show photocatalytic currents far shy of their theoretical maximum. Numerous strategies have been developed to improve their activity, which include nanostructuring, the use of surface cocatalysts, pacifying surface states, and forming heterojunction architectures. This review focuses on the use of TiO 2 , α-Fe 2 O 3 , BiVO 4, and WO 3 as photoanodes for water oxidation and studies that probe charge carrier dynamics. Emphasis is placed on evaluation of electrodes under operating conditions. During this review, we will discuss each metal oxide in turn and use these studies of charge carrier dynamics to build an inclusive and complimentary picture of the processes that occur during water oxidation. There will be a general view on how changes in material structure impact charge carrier dynamics and the kinetics of water oxidation." @default.
- W2599523653 created "2017-04-07" @default.
- W2599523653 creator A5032592689 @default.
- W2599523653 creator A5079316630 @default.
- W2599523653 creator A5086035043 @default.
- W2599523653 date "2017-01-01" @default.
- W2599523653 modified "2023-09-25" @default.
- W2599523653 title "Charge Carrier Dynamics in Metal Oxide Photoelectrodes for Water Oxidation" @default.
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