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- W2599691845 abstract "Transamination of [Co{N(SiMe3 )2 }2 ]2 with C6 H4 (NHSiiPr3 )2 gave the centrosymmetric trinuclear [{Coter N(SiMe3 )2 (μ-η-[o-C6 H4 (κNSiiPr3 )2 ])}2 Coint ] (1) (Coter , Coint =terminal, internal Co, respectively), with 3-coordinate Coter , and Coint sandwiched between the o-phenylenes of the two ligands; experimental and computational data support CoII centres and ditopic o-amido-imino-cyclohexen-allyl ligands; magnetic studies reveal intermetallic ferromagnetic interactions and single-molecule magnet (SMM) character. One-electron reduction of 1 yielded the salt [K(18-crown-6)(THF)2 ][{Coter N(SiMe3 )2 (μ-η-[o-C6 H4 (κNSiiPr3 )2 ])}2 Coint ] (4) with the anion isostructural to 1. The centrosymmetric Fe complex [{Feter N(SiMe3 )2 (μ-η-[o-C6 H4 (κNSiiPr3 )2 ])}2 Feint ] (5), analogous to 1, was also obtained." @default.
- W2599691845 created "2017-04-07" @default.
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- W2599691845 date "2017-04-19" @default.
- W2599691845 modified "2023-10-05" @default.
- W2599691845 title "Linear, Trinuclear Cobalt Complexes with <i>o</i> -Phenylene-bis-Silylamido Ligands" @default.
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- W2599691845 doi "https://doi.org/10.1002/chem.201700496" @default.
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