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- W2600160918 abstract "Ambient-pressure X-ray photoelectron spectroscopy (APXPS) has contributed greatly to a wide range of research fields, including environmental science [1 H. Bluhm, Journal of Electron Spectroscopy and Related Phenomena 177, 71–84 (2010).[Crossref], [Web of Science ®] , [Google Scholar]], catalysis [2 D.E. Starr et al., Chemical Society Reviews 42, 5833–5857 (2013).[Crossref], [PubMed], [Web of Science ®] , [Google Scholar]], and electrochemistry [3 E.J. Crumlin, H. Bluhm, and Z. Liu, Journal of Electron Spectroscopy and Related Phenomena 190, 84–92 (2013).[Crossref], [Web of Science ®] , [Google Scholar]], to name a few. The use of this technique at synchrotron facilities primarily focused on probing the solid/gas interface; however, it quickly advanced to the probing of liquid/vapor interfaces [4 D.E. Starr et al., Physical Chemistry Chemical Physics 10, 3093–3098 (2008).[Crossref], [PubMed], [Web of Science ®] , [Google Scholar], 5 M.A. Brown et al., Physical Chemistry Chemical Physics 10, 4778–4784 (2008).[Crossref], [PubMed], [Web of Science ®] , [Google Scholar]] and solid/liquid interfaces through an X-ray-transparent window [6 J. Kraus et al., Nanoscale 6, 14394–14403 (2014).[Crossref], [PubMed], [Web of Science ®] , [Google Scholar]–8 T. Masuda et al., Appl Phys Lett 103 (2013).[Crossref], [Web of Science ®] , [Google Scholar]]. Most recently, combining APXPS with “Tender” X-rays (~2.5 keV to 8 keV) on beamline 9.3.1 at the Advanced Light Source in Lawrence Berkeley National Laboratory (which can generate photoelectrons with much longer inelastic mean free paths) has enabled us to probe the solid/liquid interface without needing a window [9 S. Axnanda et al., Scientific Reports 5 (2015).[Crossref], [PubMed], [Web of Science ®] , [Google Scholar]]. This innovation allows us to probe interfacial chemistries of electrochemically controlled solid/liquid interfaces undergoing charge transfer reactions [9 S. Axnanda et al., Scientific Reports 5 (2015).[Crossref], [PubMed], [Web of Science ®] , [Google Scholar]]. These advancements have transitioned APXPS from a traditional surface science tool to an essential interface science technique." @default.
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- W2600160918 date "2017-03-04" @default.
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- W2600160918 title "Ambient-Pressure X-ray Photoelectron Spectroscopy to Characterize the Solid/Liquid Interface: Probing the Electrochemical Double Layer" @default.
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- W2600160918 doi "https://doi.org/10.1080/08940886.2017.1289806" @default.
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