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- W2600678307 abstract "Fe2O3 nanoparticles with a mean size of ∼1 nm were evenly distributed inside the mesoporous Al2O3 with a diameter of ∼1 mm using temperature-regulated chemical vapor deposition (TR-CVD), in which Fe(Cp)2 vapor and air were use as metal precursor and oxidizing agent, respectively. For comparison, NiO/Al2O3 was prepared by a similar method using Ni(Cp)2 vapor as Ni precursor, and the resulting structure showed NiO nanoparticles decorating only the shell part of the Al2O3 bead with a shell depth of ∼50 μm. After post-annealing of these samples under air at 450–750 °C, these structures were used as catalysts for oxidation of toluene in the reaction temperature range of 150–350 °C. Fe2O3/Al2O3 showed significantly higher catalytic activity than NiO-based catalysts, which can be attributed to the unique structure of Fe2O3/Al2O3, i.e., very small catalytically active nanoparticles are distributed inside the entire structure of the mesoporous supporting material. 100% conversion of toluene into CO2 with a long-term stability of the catalytic activity was realized at 350 °C using Fe2O3/Al2O3 under both dry and humid conditions with a toluene concentration of 10,000 ppm in the feed gas. It is worth noting that the unique structure of the Fe2O3/Al2O3 is stable after air-post-annealing at 750 °C. Our Fe2O3/Al2O3 catalysts are active for toluene oxidation, and stable upon annealing at high temperature, showing that one can use our Fe2O3/Al2O3 as a component of catalytic converter of harmful volatile organic compounds." @default.
- W2600678307 created "2017-04-07" @default.
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- W2600678307 date "2017-10-01" @default.
- W2600678307 modified "2023-10-14" @default.
- W2600678307 title "Activity of catalysts consisting of Fe 2 O 3 nanoparticles decorating entire internal structure of mesoporous Al 2 O 3 bead for toluene total oxidation" @default.
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- W2600678307 doi "https://doi.org/10.1016/j.cattod.2017.03.023" @default.
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