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- W2600785110 abstract "Amorphization in metal-organic framework materials initiated by the collapsed crystal offers new access to glasses; however, the understanding of such glasses remains to be clarified. Here, we studied the glass transition thermodynamics and kinetics in a zeolitic imidazolate framework ZIF-4 utilizing enthalpy relaxation measurements. The calorimetric glass transition profile and relaxation behaviors in ZIF-4 are found to reproduce the basic features and correlations manifested by conventional melt-quenched glasses. A comparison with various melt-quenched glasses suggests that the low fragility of ZIF-4 is ascribed to the low thermal-pressure coefficient due to the directional tetrahedral bond, partly leading to the low vibrational entropy in the melt-crystal entropy difference." @default.
- W2600785110 created "2017-04-07" @default.
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- W2600785110 date "2017-03-28" @default.
- W2600785110 modified "2023-10-18" @default.
- W2600785110 title "Communication: Enthalpy relaxation in a metal-organic zeolite imidazole framework (ZIF-4) glass-former" @default.
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- W2600785110 doi "https://doi.org/10.1063/1.4979352" @default.
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