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- W2601523367 abstract "Transitions between different charge density wave (CDW) states in quasi-two-dimensional materials may be accompanied also by changes in the inter-layer stacking of the CDW. Using MeV ultrafast electron diffraction, the out-of-plane stacking order dynamics in the quasi-two-dimensional dichalcogenide 1T-TaS$_2$ is investigated for the first time. From the intensity of the CDW satellites aligned around the commensurate $l$ = 1/6 characteristic stacking order, it is found out that this phase disappears with a 0.5 ps time constant. Simultaneously, in the same experiment, the emergence of the incommensurate phase, with a slightly slower 2.0 ps time constant, is determined from the intensity of the CDW satellites aligned around the incommensurate $l$ = 1/3 characteristic stacking order. These results might be of relevance in understanding the metallic character of the laser-induced metastable hidden state recently discovered in this compound." @default.
- W2601523367 created "2017-04-07" @default.
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- W2601523367 date "2017-07-01" @default.
- W2601523367 modified "2023-10-17" @default.
- W2601523367 title "Stacking order dynamics in the quasi-two-dimensional dichalcogenide 1<i>T</i>-TaS<sub>2</sub> probed with MeV ultrafast electron diffraction" @default.
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- W2601523367 doi "https://doi.org/10.1063/1.4982918" @default.
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