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• W2605643721 abstract "Different crystal facets with different surface atomic configurations and physical/chemical properties will have distinct electrochemical performances during their surface/near-surface redox reactions, and it is important to realize the controllable synthesis of high active surfaces for electrode materials. Herein, using first-principles calculations, the electrochemical performances of different surfaces of β-MnO2 were investigated. Higher surface adsorption pseudocapacitance and lower ion diffusion barrier from the surface to the near surface make the {001} surface of β-MnO2 superior to other surfaces when acting as an electrode material. Moreover, β-MnO2 with a large percentage of the {001} surface was predicted to be obtained through surface F-termination. F-termination decreases the surface energy of the {001} surface while suppressing the growth of {110} surface, which demonstrated as the surface with a much lower electrochemical performance. This work might provide a feasible strategy to synthesize anticipated surfaces with a high electrochemical performance for transition metal oxides." @default.
• W2605643721 created "2017-04-28" @default.
• W2605643721 creator A5008214844 @default.
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• W2605643721 date "2017-04-20" @default.
• W2605643721 modified "2023-10-15" @default.
• W2605643721 title "Promoted Electrochemical Performance of β-MnO₂ through Surface Engineering" @default.
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• W2605643721 doi "https://doi.org/10.1021/acsami.6b14601" @default.
• W2605643721 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/28397492" @default.
• W2605643721 hasPublicationYear "2017" @default.
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