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- W2605966273 abstract "Functionalized polypropylene with hydroxyl group (PPOH) nanocomposites with varying chemical structures in filler-matrix interfaces were examined by rheo-optical near-infrared measurements combined with two-dimensional correlation spectroscopy, to provide a better understanding of the reinforcement mechanism of nanocomposites. PPOH nanocomposites were fabricated by melt-mixing (i) silica nanospheres (SNS) and (ii) SNS modified with surfactant (mSNS). The decrease in the asynchronous correlation intensity from PPOH to SNS/PPOH indicated that the tensile deformation of amorphous and crystalline occurred simultaneously. These observations implied that the high interfacial adhesion between filler and matrix restricted the deformation of amorphous. This mechanism seems to contribute to the improvement in mechanical strength of the composite. The asynchronous correlation intensity of mSNS/PPOH was higher than that of SNS/PPOH, indicating that a certain level of deformation of the amorphous was allowed. It is therefore likely that the surface modification of SNS prevented filler-matrix interactions, leading to relatively low tensile strength of mSNS/PPOH. Thus, the techniques based on NIR spectroscopy clarify the effects of the filler-matrix interfacial adhesion of nanocomposites on the behavior of the crystalline and amorphous components during tensile testing, and may be generally applicable to evaluate filler-matrix adhesion behavior of a wide range of polymer nanocomposite systems." @default.
- W2605966273 created "2017-04-28" @default.
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- W2605966273 date "2017-07-01" @default.
- W2605966273 modified "2023-10-17" @default.
- W2605966273 title "Reinforcement mechanism of functionalized polypropylene containing hydroxyl group nanocomposites studied by rheo-optical near-infrared spectroscopy" @default.
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- W2605966273 doi "https://doi.org/10.1016/j.eurpolymj.2017.04.032" @default.
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