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- W2606562005 abstract "The non-radiative relaxation dynamics of pyrrole have been investigated using time-resolved photoelectron spectroscopy and quantum dynamics simulations. Following excitation of the A2(11πσ∗) state, we observe population flow out of the Franck-Condon region on a ≲50 fs timescale. Following excitation of the B2(21ππ∗) state, we observe population being transferred to the A2(11πσ∗) state on a <50 fs timescale and subsequently out of the Franck-Condon region, also on a <50 fs timescale. Quantum dynamics calculations suggest that population is transferred from the B2(21ππ∗) state through the A2(1π3pz) state to the B1(21πσ∗) state before being transferred to the A2(11πσ∗) state." @default.
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- W2606562005 date "2017-09-01" @default.
- W2606562005 modified "2023-10-08" @default.
- W2606562005 title "Non-radiative relaxation dynamics of pyrrole following excitation in the range 249.5–200 nm" @default.
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- W2606562005 doi "https://doi.org/10.1016/j.cplett.2017.04.035" @default.
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