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- W2606576384 abstract "Selective ion-exchange with zeolites has been considered as one of the most promising means to remove a radioactive isotope of cesium, 137Cs, present in low concentration in seawater. However, there has been no report on the fundamental structure–property relation of zeolite-based Cs ion-exchangers. In this study, we investigate the origin of the selectivity of the radioactive cesium isotope in zeolite frameworks using zeolite A (LTA) as a model system. We prepared seven single crystals of fully dehydrated and partially cesium exchanged Zeolite A (LTA) with different Cs+/Na+ ratios. Their single-crystal synchrotron X-ray diffraction experiments revealed the significant differences in the degree of exchange and the site selectivity of Cs+ ions depending on the initial Cs+ concentrations in given ion exchange solutions. The degree of Cs+-ion exchange increases from 15.8 to 44.2% as the initial Cs+ concentration increases and the Na+ content decreases. In addition, it was found that Cs+ ions are energeticall..." @default.
- W2606576384 created "2017-04-28" @default.
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- W2606576384 date "2017-05-04" @default.
- W2606576384 modified "2023-10-16" @default.
- W2606576384 title "Selective Removal of Radioactive Cesium from Nuclear Waste by Zeolites: On the Origin of Cesium Selectivity Revealed by Systematic Crystallographic Studies" @default.
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- W2606576384 doi "https://doi.org/10.1021/acs.jpcc.7b02432" @default.
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