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• W2606742148 abstract "Abstract Historically, it is believed that crystalline uraninite, produced via the abiotic reduction of hexavalent uranium (U (VI) ) is the dominant reduced U species formed in low-temperature uranium roll-front ore deposits. Here we show that non-crystalline U (IV) generated through biologically mediated U (VI) reduction is the predominant U (IV) species in an undisturbed U roll-front ore deposit in Wyoming, USA. Characterization of U species revealed that the majority (∼58-89%) of U is bound as U (IV) to C-containing organic functional groups or inorganic carbonate, while uraninite and U (VI) represent only minor components. The uranium deposit exhibited mostly 238 U-enriched isotope signatures, consistent with largely biotic reduction of U (VI) to U (IV) . This finding implies that biogenic processes are more important to uranium ore genesis than previously understood. The predominance of a relatively labile form of U (IV) also provides an opportunity for a more economical and environmentally benign mining process, as well as the design of more effective post-mining restoration strategies and human health-risk assessment." @default.
• W2606742148 created "2017-04-28" @default.
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• W2606742148 date "2017-06-01" @default.
• W2606742148 modified "2023-10-02" @default.
• W2606742148 title "Biogenic non-crystalline U(IV) revealed as major component in uranium ore deposits" @default.
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• W2606742148 doi "https://doi.org/10.1038/ncomms15538" @default.
• W2606742148 hasPubMedCentralId "https://www.ncbi.nlm.nih.gov/pmc/articles/5461479" @default.
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