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- W2607223601 abstract "Abstract Ordered mesoporous silica materials based on nickel and other elements have been extensively studied because controlling the size of metal nanoparticles is an effective method to tune the superficial physicochemical process. Neodymium (Nd)-promoted mesoporous silica xNdMS (x: molar ratio of Nd/Si = 0.01, 0.02, 0.04, 0.06) were prepared through a sol–gel strategy. Nickel-based catalysts with high dispersion by using xNdMS as supports were investigated for methane reforming with carbon dioxide and/or oxygen to produce syngas. xNdMS supports and nickel catalysts were examined by combining textural, structural, local and surface information. The characterization results showed that Nd was successfully incorporated into the mesoporous framework of MS and Nd was beneficial to improve the metal dispersion. All Nd-promoted Ni/MS catalysts were effective for the methane reforming reaction. Ni/0.04NdMS catalyst exhibited the highest initial catalytic activity during 12 h time on stream, which was attributed to its high metal dispersion, more basic sites and the strengthened nickel-support interaction. The readily deactivation and poorest catalytic activity of Ni/MS catalyst were due to the serious oxidation of metallic nickel under reaction medium." @default.
- W2607223601 created "2017-04-28" @default.
- W2607223601 creator A5014740040 @default.
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- W2607223601 date "2017-04-01" @default.
- W2607223601 modified "2023-10-17" @default.
- W2607223601 title "Catalytic performance and characterization of Neodymium-containing mesoporous silica supported nickel catalysts for methane reforming to syngas" @default.
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- W2607223601 doi "https://doi.org/10.1016/j.ijhydene.2017.03.159" @default.
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