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• W2607662919 endingPage "5141" @default.
• W2607662919 startingPage "5133" @default.
• W2607662919 abstract "Recrystallization behaviors of water sorbed into four poly(meth)acrylates, poly(2-methoxyethyl acrylate), poly(tetrahydrofurfuryl acrylate), poly(methyl acrylate), and poly(methyl methacrylate), are investigated by variable-temperature mid-infrared (VT-MIR) spectroscopy and molecular dynamics (MD) simulation. VT-MIR spectra demonstrate that recrystallization temperatures of water sorbed into the polymers are positively correlated with their glass-transition temperatures reported previously. The present MD simulation shows that a lower-limit temperature of the diffusion for the sorbed water and the glass-transition temperatures of the polymers also have a positive correlation, indicating that the recrystallization is controlled by diffusion mechanism rather than reorientation mechanism. Detailed molecular processes of not only recrystallization during rewarming but also crystallization during cooling and hydrogen-bonding states of water in the polymers are systematically analyzed and discussed." @default.
• W2607662919 created "2017-05-05" @default.
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• W2607662919 date "2017-05-10" @default.
• W2607662919 modified "2023-10-18" @default.
• W2607662919 title "Diffusion-Controlled Recrystallization of Water Sorbed into Poly(meth)acrylates Revealed by Variable-Temperature Mid-Infrared Spectroscopy and Molecular Dynamics Simulation" @default.
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• W2607662919 doi "https://doi.org/10.1021/acs.jpcb.7b01824" @default.
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• W2607662919 hasPublicationYear "2017" @default.
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