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• W2608587425 abstract "Abstract Positron annihilation lifetime spectroscopy in high-measurements statistics supported by ab initio quantum chemical modeling developed within cation-interlinking network cluster approach were used to examine compositional peculiarities of free-volume evolution in Se-rich As-Se glasses. Existence of some anomalies in the studied glasses observed as jump in the defect-related positron lifetime near average coordination Z ≈ 2.33 and strong growing trend approaching Z = 2.40 is justified. These features correspond to evolution of glassy network due to free-volume elements based on solid angle free of bond charge associated with Se atoms in a vicinity of heteropolar chemical bonds. The results are explained within structural models of optimized network of As-Se glasses composed of AsSe3/2 pyramids interlinked by variable-length Se-chains." @default.
• W2608587425 created "2017-05-05" @default.
• W2608587425 creator A5018345581 @default.
• W2608587425 date "2017-07-01" @default.
• W2608587425 modified "2023-09-27" @default.
• W2608587425 title "Compositional anomalies in Se-rich As-Se glass-forming system as revealed from positron annihilation lifetime spectroscopy and ab initio cluster modeling" @default.
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• W2608587425 doi "https://doi.org/10.1016/j.commatsci.2017.04.022" @default.
• W2608587425 hasPublicationYear "2017" @default.
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