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- W2610281044 abstract "In this work, a series of Ni-Mg-Al catalysts with different Mg molar contents were prepared via a co-precipitation method. These catalysts were used for the biogas reforming of carbon dioxide (BRCD) for syngas production. The influence of Mg molar contents on the catalyst structure and catalytic performance was investigated. During the 60 h stability test at 750 °C, all of the Mg-promoted catalysts presented a higher catalytic activity and better stability in comparison with the catalyst without Mg loading. The NM10A sample with 10 mol% Mg loading displayed the highest CH4 and CO2 conversion of 86.9% and 90.8%, respectively. The catalysts were characterized by N2 adsorption-desorption analysis, XRD, H2-TPR, CO2-TPD, TEM and TGA techniques. It was found that the addition of Mg inhibited the sintering of Ni particle and increased the catalyst basicity. Consequently this suppressed the coke deposition and improved the catalytic activity. The NM10A catalyst possessed the most basic sites, which caused a minimum amount carbon to be deposited on the catalyst and allowed for the best catalytic activity. The obvious increase of the Ni metal size and the severe coke deposition resulted in the deactivation of the NM0A catalyst." @default.
- W2610281044 created "2017-05-12" @default.
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- W2610281044 date "2017-07-01" @default.
- W2610281044 modified "2023-10-17" @default.
- W2610281044 title "Biogas reforming of carbon dioxide to syngas production over Ni-Mg-Al catalysts" @default.
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- W2610281044 doi "https://doi.org/10.1016/j.mcat.2017.04.032" @default.
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