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- W2610693789 abstract "Abstract In this study, the hybrid cross-linked membranes consisting of amino functionalized polyhedral oligomeric silsesquioxanes (POSS-NH 2 ) nanoparticles and CO 2 -philic poly(ethylene oxide) (PEO) are prepared via a facile one-step method. Porous POSS-NH 2 with abundant amino groups in the polymer matrix generates a compatible interface between the polymer matrix and nanoparticles, enhancing the CO 2 permeability. Due to the synergetic effects of nanoporous POSS-NH 2 and CO 2 -philic PEO, the hybrid cross-linked membranes exhibit excellent CO 2 permeability and selectivity. A high CO 2 permeability of 385.8 Barrer in the hybrid cross-linked membrane is achieved, which is 242% of that of pristine cross-linked membrane. The gas transport performance is explained based on the solution-diffusion mechanism and diffusion coefficient and solubility coefficient are evaluated. Furthermore, thermodynamics is explored to clarify the enhancement of gas transport performance in hybrid cross-linked membranes. The gas permeability of CH 4 , H 2 , N 2 , and CO 2 continuously improved with temperatures. The activation energies of CH 4 , N 2 , H 2 and CO 2 in hybrid cross-linked membranes are typically lower than those in the pristine cross-linked membrane, which results in the fast transportation of gases. Our developed membranes have demonstrated a promising prospect for sustainable CO 2 separations." @default.
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- W2610693789 date "2017-06-01" @default.
- W2610693789 modified "2023-10-15" @default.
- W2610693789 title "Effects of amino functionalized polyhedral oligomeric silsesquioxanes on cross-linked poly(ethylene oxide) membranes for highly-efficient CO 2 separation" @default.
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- W2610693789 doi "https://doi.org/10.1016/j.cherd.2017.04.025" @default.
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