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• W2611104465 endingPage "11961" @default.
• W2611104465 startingPage "11956" @default.
• W2611104465 abstract "CsPbBr3 nanocrystals passivated with short molecular ligands and deposited on a substrate were annealed from room temperature to 400 °C in inert atmosphere. Chemical, structural, and morphological transformations were monitored in situ and ex situ by different techniques, while optoelectronic properties of the film were also assessed. Annealing at 100 °C resulted in a 1 order of magnitude increase in photocurrent and photoresponse as a result of partial sintering of the NCs and residual solvent evaporation. Beyond 150 °C the original orthorhombic NCs were partially transformed into tetragonal CsPb2Br5 crystals, due to the desorption of weakly bound propionic acid ligands. The photocurrent increased moderately until 300 °C although the photoresponse became slower as a result of the formation of surface trap states. Eventually, annealing beyond 350 °C removed the strongly bound butylamine ligands and reversed the transition to the original orthorhombic phase, with a loss of photocurrent due to the numerous defects induced by the stripping of the passivating butylamine." @default.
• W2611104465 created "2017-05-12" @default.
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• W2611104465 date "2017-05-03" @default.
• W2611104465 modified "2023-10-12" @default.
• W2611104465 title "From CsPbBr₃ Nano-Inks to Sintered CsPbBr₃–CsPb₂Br₅ Films via Thermal Annealing: Implications on Optoelectronic Properties" @default.
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• W2611104465 doi "https://doi.org/10.1021/acs.jpcc.7b03389" @default.
• W2611104465 hasPubMedCentralId "https://www.ncbi.nlm.nih.gov/pmc/articles/6284206" @default.
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