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- W2612731936 abstract "Very large molecular two- and three-photon absorption cross-sections are achieved by appending ligated bis(diphosphine)ruthenium units to oligo(p-phenyleneethynylene) (OPE)-based “stars” with arms up to 7 phenyleneethynylene (PE) units in length. Extremely large three- and four-photon absorption cross-sections, through the telecommunications wavelengths range and beyond, are obtained for these complexes upon optimizing OPE length and the ruthenium-coordinated peripheral ligand. Multi-photon absorption (MPA) cross-sections are optimized with stars possessing arms 2 PE units in length. Peripheral ligand variation modifies MPA merit and, in particular, 4-nitrophenylethynyl ligand incorporation enhances maximal MPA values and “switches on” four-photon absorption (4PA) in these low molecular-weight complexes. The 4-nitrophenylethynyl-ligated 2PE-armed star possesses a maximal four-photon absorption cross-section of 1.8×10−108 cm8 s3 at 1750 nm, and significant MPA activity extending beyond 2000 nm." @default.
- W2612731936 created "2017-05-19" @default.
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- W2612731936 date "2017-06-01" @default.
- W2612731936 modified "2023-10-03" @default.
- W2612731936 title "Stellar Multi‐Photon Absorption Materials: Beyond the Telecommunication Wavelength Band" @default.
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- W2612731936 doi "https://doi.org/10.1002/chem.201702039" @default.
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