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• W2613355190 abstract "Molecular semiconductors offer intriguing electronic properties. In particular, singlet-exciton fission, the nonradiative decay of one singlet exciton into two triplet excitons effectively doubles the amount of carriers available for, e.g., photovoltaic current generation, thereby effectively surpassing the Shockley-Queisser-limit. An efficient use of singletexciton fission in actual devices, however, requires a detailed understanding of the decay dynamics in donor-acceptor heterostructures. We present a quantitative study on model single-crystalline perfluropentacene at cryogenic temperature and related heterostructures to reveal the intricate interplay between singlet-exciton fission and the nanoscopic molecular arrangement, the role of charge-transfer into and out of molecular systems and discuss the potential for functionalizing inorganic semiconductors. Finally, the potential implications in heterosystems and for functionalization of inorganic semiconductor devices are discussed." @default.
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• W2613355190 date "2017-05-08" @default.
• W2613355190 modified "2023-09-23" @default.
• W2613355190 title "Towards exploitation of singlet-exciton fission in organic crystals and potential integration with inorganic semiconductors" @default.
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• W2613355190 doi "https://doi.org/10.1117/12.2278673" @default.
• W2613355190 hasPublicationYear "2017" @default.
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