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• W2615778669 startingPage "2901" @default.
• W2615778669 abstract "A metal-catalyst-free, mild, and efficient synthetic protocol for polycyclic 1,4-benzodiazepines via cascade [5 + 2]/[2 + 2] cycloadditions between pyridinium zwitterions and arynes is reported. Mechanistic experiments revealed that pyridinium zwitterions act as 1,5-dipoles in [5 + 2] cycloadditions with arynes for the construction of 1,4-benzodiazepines, which further undergo [2 + 2] cycloaddition resulting in the one-pot formation of one C–N bond and three C–C bonds." @default.
• W2615778669 created "2017-05-26" @default.
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• W2615778669 date "2017-05-18" @default.
• W2615778669 modified "2023-10-10" @default.
• W2615778669 title "Synthesis of Fused Polycyclic 1,4-Benzodiazepines via Metal-Free Cascade [5 + 2]/[2 + 2] Cycloadditions" @default.
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• W2615778669 doi "https://doi.org/10.1021/acs.orglett.7b01137" @default.
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