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• W2616057184 abstract "Optical initialization of the negatively charged nitrogen-vacancy (NV${}^{ensuremath{-}}$) center in diamond makes it one of the best candidates for realization of addressable spins in the solid state for quantum computing and other studies. However, its exact mechanism was not clear. We show that exact diagonalization of a many-electron Hamiltonian with parameters derived from ab initio GW calculations puts strong constraints on the mechanism. The energy surfaces of the low-energy many-body states and the relaxation processes of photoexcitation responsible for the optical initialization are calculated. Intersystem crossings are shown to be essential." @default.
• W2616057184 created "2017-05-26" @default.
• W2616057184 creator A5007422862 @default.
• W2616057184 creator A5040814439 @default.
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• W2616057184 date "2012-07-20" @default.
• W2616057184 modified "2023-09-25" @default.
• W2616057184 title "Mechanism for optical initialization of spin in NV<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML display=inline><mml:msup><mml:mrow /><mml:mo>−</mml:mo></mml:msup></mml:math>center in diamond" @default.
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• W2616057184 doi "https://doi.org/10.1103/physrevb.86.041202" @default.
• W2616057184 hasPublicationYear "2012" @default.
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