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• W2616155844 abstract "We report a unique example of utilizing unprotected amino acids for benzylic C–H fluorination via a radical process. α-Aminoalkyl radicals are readily generated via oxidative decarboxylation of unprotected amino acids using a simple silver(I) catalyst and Selectfluor, which serves as both a mild oxidant and source of electrophilic fluorine. Mechanistic investigation shows that coordination of the unprotected amino acid plays a crucial role in lowering the oxidation potential of Ag(I), enabling oxidation under mild conditions. Mono- or difluorination is possible by controlling the stoichiometry of amino acid and fluorine source." @default.
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• W2616155844 date "2017-05-17" @default.
• W2616155844 modified "2023-10-15" @default.
• W2616155844 title "Radical C–H Fluorination Using Unprotected Amino Acids as Radical Precursors" @default.
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• W2616155844 doi "https://doi.org/10.1021/acs.orglett.7b01188" @default.
• W2616155844 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/28513162" @default.
• W2616155844 hasPublicationYear "2017" @default.
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