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- W2616367498 abstract "9,10-Anthraquinone-2,7-disulfonic acid (AQDS) is considered a benchmark active material for aqueous organic redox flow batteries. At low concentration, AQDS demonstrates two-electron transfer at near ideal electrochemical reversibility; however, at higher concentration, AQDS displays more complex behavior presumably due to the emergence of intermolecular reactions. Here, we systematically examine the electrochemical and physical properties of AQDS solutions using a suite of electrochemical, analytical, and spectroscopic techniques. Depending on the AQDS pretreatment, concentration, solution pH, and electrolyte composition, coupled chemical and electrochemical reactions lead to different charge storage capabilities. To elucidate the underlying cause of these differences, we performed various pretreatments of AQDS, examined chemical speciation by NMR, and investigated the corresponding electrochemical properties through cyclic voltammetry and bulk electrolysis. In all cases, reversible intermolecular dimeri..." @default.
- W2616367498 created "2017-05-26" @default.
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- W2616367498 date "2017-06-01" @default.
- W2616367498 modified "2023-10-14" @default.
- W2616367498 title "Concentration-Dependent Dimerization of Anthraquinone Disulfonic Acid and Its Impact on Charge Storage" @default.
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- W2616367498 doi "https://doi.org/10.1021/acs.chemmater.7b00616" @default.
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