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- W2617163341 abstract "Controlling morphological order of conjugated polymers over mesoscopic and microscopic scales could yield critical improvements in the performance of organic electronics. Here, we utilize a multimodal apparatus allowing for controlled solvent vapor annealing and simultaneous wide-field epifluorescence microscopy to demonstrate bottom-up growth of morphologically ordered anisotropic aggregates prepared from single poly(2-methoxy-5-(2-ethylhexyloxy)-1,4-phenylenevinylene) (MEH-PPV) chains, with length scales controllable from tens of nanometers to several micrometers. Preparation of micrometer-scale fiber aggregates that interconnect to form spanning networks is also demonstrated. We quantify aggregate physical and optical anisotropy, degree of quenching, and exciton diffusion characteristics as a function of aggregate size. The demonstration of controlled preparation of highly anisotropic aggregates provides a path for controlled postprocessing of organic thin films at length scales relevant to the operation of devices." @default.
- W2617163341 created "2017-06-05" @default.
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- W2617163341 date "2017-06-19" @default.
- W2617163341 modified "2023-09-24" @default.
- W2617163341 title "Highly Anisotropic Conjugated Polymer Aggregates: Preparation and Quantification of Physical and Optical Anisotropy" @default.
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- W2617163341 doi "https://doi.org/10.1021/acs.jpcc.7b02257" @default.
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