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• W2617503012 abstract "The combined contamination of arsenic (As) and fluoride (F) in groundwater poses severe health risks. However, little information is available on the simultaneous removal of As(III)&F, not to mention their competition behaviors. Hence, we investigated the characteristics of competitive adsorption between As(III) and F onto the surface of Mn-Al binary oxides (MABO). The co-adsorption behaviors of As(III/V)&F, including isotherm and kinetic characteristics, were influenced by As speciations, solution pH, and Mn/Al molar ratios. With sequential addition of As(V)&F, the non-exchangeable fraction for each ion was approximately equal to their initially adsorbed amounts, respectively. Moreover, the adsorption amount of As(V) or F in the rapid reaction stage was attributed to the surface complexation formation. By contrast, when As(III) and F were adsorbed sequentially, the As(III) molecules adsorbed in the rapid reaction stage was more vulnerable and easily replaced by F ions. Additionally, the non-exchangeable fraction for adsorbed As was mainly As(V), which was converted from As(III) via redox reactions. These results suggested that the competition between As(III) and F is quite different with that between As(V) and F onto MABO surfaces. Furthermore, F complexation formation not only inhibits the adsorption of As(III), but also suppresses the oxidative reactivity of MABO." @default.
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• W2617503012 date "2017-09-01" @default.
• W2617503012 modified "2023-10-17" @default.
• W2617503012 title "Competitive adsorption behaviors of arsenite and fluoride onto manganese-aluminum binary adsorbents" @default.
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• W2617503012 doi "https://doi.org/10.1016/j.colsurfa.2017.05.039" @default.
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