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• W2617850923 abstract "Wavefunctions for large electron numbers suffer from an exponential growth of the Hilbert space which is required for their description. In fact, as pointed out by W. Kohn, for electron numbers (N > N_0) where (N_0 approx 10^3) they become meaningless (exponential wall problem). Nevertheless, despite of the enormous successes of density functional theory, one would also like to develop electronic structure calculations for solids based on wavefunctions. This is possible if one defines the latter in Liouville space with a cumulant metric instead in Hilbert space. The cluster expansion of the free energy of a classical monatomic gas makes it transparent why cumulants are very well suited also for electronic structure calculations." @default.
• W2617850923 created "2017-06-05" @default.
• W2617850923 creator A5069172628 @default.
• W2617850923 date "2018-01-01" @default.
• W2617850923 modified "2023-09-27" @default.
• W2617850923 title "Wavefunctions for Large Electronic Systems" @default.
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• W2617850923 doi "https://doi.org/10.1007/978-3-319-72374-7_8" @default.
• W2617850923 hasPublicationYear "2018" @default.
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