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- W2619573705 abstract "Abstract In this work, we established catalytic asymmetric [4+1] cyclization of ortho ‐quinone methides ( o ‐QMs) with 3‐chlorooxindoles and a catalytic asymmetric domino oxidation/[4+1] cyclization reaction of 2‐alkylphenols with 3‐chlorooxindoles, which constructed a spirooxindole‐based 2,3‐dihydrobenzofuran scaffold in good yield (up to 97%), with excellent diastereoselectivity (up to >95:5 dr ) and high enantioselectivity (up to 99% ee ). This work is not only the first highly enantioselective [4+1] cyclization of o ‐QMs but has also realized the first catalytic asymmetric domino [4+1] cyclization of o ‐QMs. In addition, both of the reactions provide efficient stereoselective methods for constructing spirooxindole‐based 2,3‐dihydrobenzofuran scaffolds with optical purity. magnified image" @default.
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- W2619573705 date "2017-06-19" @default.
- W2619573705 modified "2023-10-15" @default.
- W2619573705 title "Catalytic Asymmetric [4+1] Cyclization of <i>ortho</i> -Quinone Methides with 3-Chlorooxindoles" @default.
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- W2619573705 doi "https://doi.org/10.1002/adsc.201700487" @default.
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