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- W2620495564 endingPage "8864" @default.
- W2620495564 startingPage "8860" @default.
- W2620495564 abstract "The first regio-, diastereo-, and enantioselective direct Michael reaction of β,γ-unsaturated ketones with nitroolefins is enabled by Brønsted base/hydrogen-bonding bifunctional catalysis. A squaramide-substituted tertiary amine catalyzes the reaction of a broad range of β,γ-unsaturated ketones to proceed at the α-site exclusively, giving rise to adducts with two consecutive tertiary carbon stereocenters in diastereomeric ratios of up to >20:1 and enantioselectivities generally in the 90-98 % ee range." @default.
- W2620495564 created "2017-06-05" @default.
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- W2620495564 date "2017-06-20" @default.
- W2620495564 modified "2023-10-01" @default.
- W2620495564 title "Controlling the α/γ-Reactivity of Vinylogous Ketone Enolates in Organocatalytic Enantioselective Michael Reactions" @default.
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- W2620495564 doi "https://doi.org/10.1002/anie.201703764" @default.
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