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- W2620781285 abstract "Cation-π interaction is an intermolecular interaction between the face of a π system and an adjacent cation, which brings about a change in molecular dynamics of organic reactants in catalysis. In this study, a series of alkali metal cations-anchored TiO2/SiO2 hybrid catalysts were prepared based on organo-functionalized MCM-41 mesoporous silica, in order to examine the effect of cation-π interaction in heterogeneous catalysis. Immobilizing heavier alkali metal cations on surface-functionalized carboxylic acid ion-exchange sites provided a dramatic impact on diffusion properties of aromatic molecules, which led to a significant enhancement in photocatalytic degradation of phenol in water under ultraviolet light irradiation, whereas such an enhancement was not observed in degradation of cyclohexanol without π electrons. A distinct relationship was observed between the catalytic activities and adsorption energies determined by thermogravimetric analysis, which evidenced a role of the cation-π interaction as a diffusion-controlling tool in this reaction system." @default.
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- W2620781285 date "2017-05-31" @default.
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- W2620781285 title "Dramatically Enhanced Phenol Degradation on Alkali Cation-Anchored TiO2 /SiO2 Hybrids: Effect of Cation-π Interaction as a Diffusion-Controlling Tool in Heterogeneous Catalysis" @default.
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- W2620781285 doi "https://doi.org/10.1002/slct.201700708" @default.
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