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• W2621079809 abstract "High utilization and loading of sulfur in cathodes holds the key in the realization of Li-S batteries. We here synthesized a Co4N mesoporous sphere, which was made up of nanosheets, via an easy and convenient method. This material presents high affinity, speedy trapping, and absorbing capacity for polysulfides and acts as a bifunctional catalysis for sulfur redox processes; therefore it is an ideal matrix for S active material. With such a mesoporous sphere used as a sulfur host in Li-S batteries, extraordinary electrochemistry performance has been achieved. With a sulfur content of 72.3 wt % in the composite, the Co4N@S delivered a high specific discharge capacity of 1659 mAh g-1 at 0.1 C, almost reaching its theoretic capacity. Also, the battery exhibited a large reversible capacity of about 1100 mAh g-1 at 0.5 C and 1000 mAh g-1 at 1 C after 100 cycles. At a high rate of 2 C and 5 C, after 300 cycles, the discharge capacity finally stabilized at 805 and 585 mAh g-1. Even at a 94.88% sulfur content, the cathode can still deliver an extremely high specific discharge capacity of 1259 mAh g-1 with good cycle performance." @default.
• W2621079809 created "2017-06-09" @default.
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• W2621079809 date "2017-06-07" @default.
• W2621079809 modified "2023-10-15" @default.
• W2621079809 title "Co₄N Nanosheet Assembled Mesoporous Sphere as a Matrix for Ultrahigh Sulfur Content Lithium–Sulfur Batteries" @default.
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• W2621079809 doi "https://doi.org/10.1021/acsnano.7b01945" @default.
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