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• W2621130135 abstract "Full-color visible emissions are particularly crucial for applications in displays and lightings. In this work, we developed a facile room-temperature ligand-assisted supersaturated recrystallization synthesis of monodisperse, cubic structure Cs1-mFAmPbX3 (X = Cl, Br, and I or their mixtures Cl/Br and Br/I, 0 ≤ m ≤ 1) hybrid perovskite quantum dots (QDs). Impressively, cation substitution of Cs+ by FA+ was beneficial in finely tuning the band gap and in exciton recombination kinetics, improving the structural stability, and raising the absolute quantum yields up to 85%. With further assistance of anion replacement, full-spectral visible emissions in the wavelength range of 450-750 nm; narrow full width at half-maxima, and a wide color gamut, encompassing 130% of National Television System Committee television color standard, were achieved. Finally, Cs1-mFAmPbX3-polymer films retaining multicolor luminescence are prepared and a prototype white light-emitting diode device was constructed using green Cs0.1FA0.9PbBr3 and red Cs0.1FA0.9Br1.5I1.5 QDs as color converters, certainly suggesting their potential applications in the optoelectronics field." @default.
• W2621130135 created "2017-06-09" @default.
• W2621130135 creator A5004713434 @default.
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• W2621130135 date "2017-06-12" @default.
• W2621130135 modified "2023-09-23" @default.
• W2621130135 title "Full-Spectral Fine-Tuning Visible Emissions from Cation Hybrid Cs_1–<i>m</i>FA<i>_m</i>PbX₃ (X = Cl, Br, and I, 0 ≤ <i>m</i> ≤ 1) Quantum Dots" @default.
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• W2621130135 doi "https://doi.org/10.1021/acsami.7b05429" @default.
• W2621130135 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/28569064" @default.
• W2621130135 hasPublicationYear "2017" @default.
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