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• W2624973732 startingPage "21089" @default.
• W2624973732 abstract "Recent global military events, such as the conflict in Syria, have emphasized the need to find effective strategies to rapidly destroy organophosphorus-based nerve agents. In this work, we designed active site-engineered graphene oxide (GO) via polymerization (polymer bead-GOs) as organophosphorus hydrolase (OPH) mimetic hotspots for the rapid degradation of nerve agents. This hybrid catalyst has a high total turnover frequency value of 0.65 s–1 and good stability (94.8% activity maintained after 5 cycles). Mechanism investigations suggested that the high catalytic performance could be attributed to the synergistic effect among the clusters of imidazole and the presence of – COOH groups on the GO surface and Zn2+." @default.
• W2624973732 created "2017-06-23" @default.
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• W2624973732 date "2017-06-16" @default.
• W2624973732 modified "2023-10-16" @default.
• W2624973732 title "Mimicking the Active Sites of Organophosphorus Hydrolase on the Backbone of Graphene Oxide to Destroy Nerve Agent Simulants" @default.
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• W2624973732 doi "https://doi.org/10.1021/acsami.7b07770" @default.
• W2624973732 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/28621926" @default.
• W2624973732 hasPublicationYear "2017" @default.
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