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- W2625136560 abstract "Difluoroboron-β-diketones are known to exhibit very promising mechanochromic luminescence but a greater understanding of these materials and their mechanoresponsive properties is still desirable. Here we demonstrate that a combination of spectroscopic and physicochemical techniques is necessary to understand the variation of solid-state fluorescence observed under mechanical stress and thermal annealing. For this study, we decided to focus on a new fluorescent compound showing a polymorphic behavior. Our investigation on the mechanofluorochromic properties is based on a thorough spectroscopic study (steady-state and time-resolved) on powder samples and thin films deposited on paper and coverglass substrates. Three different states were identified: two crystalline states (a stable green-emissive and a metastable yellow-emissive one) and an amorphous phase (yellow orange emission). The detailed photophysical properties highlight the dynamic excimer formation processes, which can take place in the yellow-emi..." @default.
- W2625136560 created "2017-06-23" @default.
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- W2625136560 date "2017-07-19" @default.
- W2625136560 modified "2023-10-18" @default.
- W2625136560 title "Polymorphism, Mechanofluorochromism, and Photophysical Characterization of a Carbonyl Substituted Difluoroboron-β-Diketone Derivative" @default.
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- W2625136560 doi "https://doi.org/10.1021/acs.jpcc.7b01901" @default.
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