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- W2625554927 endingPage "e25414" @default.
- W2625554927 startingPage "e25414" @default.
- W2625554927 abstract "In the course of a 5 μm high-resolution infrared study of laser ablation products from carbon–sulfur targets, the ν1 vibrational mode region of linear C3S has been studied continuously from 2046 to 2065 cm−1. Besides the prominent vibrational fundamental, the region was found to feature the ν1+ν5−ν5, ν1+ν4−ν4, and even ν1+ν3−ν3 hot bands, the latter two of which were observed for the first time. Owing to the high signal-to-noise ratio obtained, the ν1 mode of C334S could also be observed in natural abundance for the first time at high spectral resolution in the infrared. At 2061 cm−1, hidden inside the R−branch of the C3S ν1 fundamental mode, a weak new band is observed which exhibits very tight line spacing and stems from a heavy both carbon and sulfur containing carrier. On the basis of high-level quantum-chemical calculations of selected carbon–sulfur chains and other carbon-rich cumulenes, this feature is attributed to the ν5 vibrational fundamental of linear SC7S, which stands for the first gas-phase spectroscopic detection of this long cumulenic chain." @default.
- W2625554927 created "2017-06-23" @default.
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- W2625554927 date "2017-06-14" @default.
- W2625554927 modified "2023-10-17" @default.
- W2625554927 title "Carbon-sulfur chains: A high-resolution infrared and quantum-chemical study of C<sub>3</sub> S and SC<sub>7</sub> S" @default.
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- W2625554927 doi "https://doi.org/10.1002/qua.25414" @default.
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