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- W2626004612 abstract "Abstract Pyrazine rings are a fundamental part of folic acid and flavine – cofactors that participate in natural electron transfer processes. Electron deficient carbon nitrides, more specifically poly(heptazine imides) (PHI), emulating the structure of these pyrazine based cofactors were synthesized polymerizing 3-amino-1,2,4-triazole-5-thiol with hexaazatriphenylene-hexacarbonitrile or hexaazatriphenylene-hexaamide at 550 °C in the eutectic mixture of KCl/LiCl. The role of hexaazatriphenylene units is 1) to create electron deficient acceptor sites in the structure of semiconductor; 2) widen the spectral coverage up to near infrared region. The significantly increased oxidative power of such doped PHI was demonstrated by running oxygen evolution from water, 0.59 μmol h −1 , under visible light irradiation in the absence of any metal co-catalyst." @default.
- W2626004612 created "2017-06-23" @default.
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- W2626004612 date "2017-11-01" @default.
- W2626004612 modified "2023-10-18" @default.
- W2626004612 title "Hexaazatriphenylene doped carbon nitrides—Biomimetic photocatalyst with superior oxidation power" @default.
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- W2626004612 doi "https://doi.org/10.1016/j.apcatb.2017.06.036" @default.
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