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• W2626292333 endingPage "23229" @default.
• W2626292333 startingPage "23222" @default.
• W2626292333 abstract "Bimetallic phosphides have attracted research interest for their synergistic effect and superior electrocatalytic activities for electrocatalytic water splitting. Herein, a MOF-derived phosphorization approach was developed to produce Ni2P-CoP bimetallic phosphides as bifunctional electrocatalysts for both hydrogen and oxygen evolution reactions (HER and OER). Ni2P-CoP shows superior electrocatalytic activities to both pure Ni2P and CoP toward HER and OER, revealing a strong synergistic effect. High-resolution transmission electron microscopy and energy dispersive X-ray spectroscopy elemental mapping analysis show that, in the sample Ni2P-CoP, the Ni2P and CoP nanoparticles with an average particle size 10-20 nm were mixed closely on the nanoscale, creating numerous Ni2P/CoP interfaces. By comparison with the sample Ni2P+CoP, in which seldom Ni2P/CoP interfaces exist, we documented that the Ni2P/CoP interface is an essential prerequisite to realize the synergistic effect and to achieve the enhanced electrocatalytic activities in Ni2P-CoP bimetallic phosphides. This finding is meaningful for designing and developing bicomponent and even multicomponent electrocatalysts." @default.
• W2626292333 created "2017-06-23" @default.
• W2626292333 creator A5014955451 @default.
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• W2626292333 date "2017-06-26" @default.
• W2626292333 modified "2023-10-17" @default.
• W2626292333 title "MOF-Derived Formation of Ni₂P–CoP Bimetallic Phosphides with Strong Interfacial Effect toward Electrocatalytic Water Splitting" @default.
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• W2626292333 doi "https://doi.org/10.1021/acsami.7b06152" @default.
• W2626292333 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/28613810" @default.
• W2626292333 hasPublicationYear "2017" @default.
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