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- W2662873333 abstract "Abstract Hybrid lead halide perovskites have emerged as high-performance photovoltaic materials with their extraordinary optoelectronic properties. In particular, the remarkable device efficiency is strongly influenced by the perovskite crystallinity and the film morphology. Here, we investigate the perovskites crystallisation kinetics and growth mechanism in real time from liquid precursor continually to the final uniform film. We utilize some advanced in situ characterisation techniques including synchrotron-based grazing incident X-ray diffraction to observe crystal structure and chemical transition of perovskites. The nano-assemble model from perovskite intermediated [PbI 6 ] 4− cage nanoparticles to bulk polycrystals is proposed to understand perovskites formation at a molecular- or nano-level. A crystallisation-depletion mechanism is developed to elucidate the periodic crystallisation and the kinetically trapped morphology at a mesoscopic level. Based on these in situ dynamics studies, the whole process of the perovskites formation and transformation from the molecular to the microstructure over relevant temperature and time scales is successfully demonstrated." @default.
- W2662873333 created "2017-06-30" @default.
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- W2662873333 date "2017-06-21" @default.
- W2662873333 modified "2023-10-12" @default.
- W2662873333 title "In situ dynamic observations of perovskite crystallisation and microstructure evolution intermediated from [PbI6]4− cage nanoparticles" @default.
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- W2662873333 doi "https://doi.org/10.1038/ncomms15688" @default.
- W2662873333 hasPubMedCentralId "https://www.ncbi.nlm.nih.gov/pmc/articles/5482054" @default.
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- W2662873333 hasPublicationYear "2017" @default.
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