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- W266424119 abstract "Bifunctional organophosphorus extractants dissolved in polar fluorinated diluents were studied, aiming at directly recovering all f-elements from the dissolver solution of spent nuclear fuel. Octyl(phenyl)-N,N-diisobutyl-carbamoyl-methylphosphine oxide (0{phi}D[iB] CMPO, 0.2-0.8 M) with 30% TBP dissolved in meta-nitrobenzotrifluoride (Fluoropole-732) dramatically expanded its extraction region without splitting out a heterogeneous third phase. Distribution ratios of U, Np, and Pu were sufficiently high for 0.4-0.8 M CMPO in this solvent system. Combination of salt-free, methylamine carbonate (MAC), citric acid, and hydrazine reagents were evaluated to obtain fractional stripping of f-elements such as TRU group and U. Static multistage extraction using artificial FBR dissolver solution supported the process feasibility. When all f-elements are extracted simultaneously, and TRU and U recovered separately with a single extraction cycle, the new extraction process, named ORGA-process, can be expected to be highly proliferation-resistant and systematically and economically advantageous. (authors)" @default.
- W266424119 created "2016-06-24" @default.
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- W266424119 date "2008-07-01" @default.
- W266424119 modified "2023-09-24" @default.
- W266424119 title "Simultaneous recovery of all actinides from spent nuclear fuel by carbamoyl-methylphosphine oxide in fluorinated diluents" @default.
- W266424119 hasPublicationYear "2008" @default.
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