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- W269743404 abstract "Decomposition of H2S with a catalytic membrane reactor was demonstrated in the lab with a ceramic membrane. Existing ceramic membrane with 40A pore size was modified with silica oxide to have a selectivity of hydrogen over nitrogen of approximately 28. Decomposition was nearly doubled of the thermodynamic equilibrium ratio (12 vs. 6.8%) at 800C with the modified membrane. Simulation study indicates up to 40% higher than equilibrium conversion could be achieved with the membrane at a higher temperature. Further, an improved membrane with a hydrogen selectivity of nearly infinite was developed with a similar modification method. A membrane like this will provide an additional enhancement in the conversion of H2S, which will be experimentally verified in the future. Another process, coupling decomposition with oxidation, was investigated with a straight tube to demonstrate the concept. Generation of SO2 was neligible. An additional 20-30% of enhancement by the concept is expected and will be experimentally verified with the modified membrane. Conceptual design on the membrane reactor utilizing existing engineering and material technology was completed for future field demonstration." @default.
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- W269743404 date "1993-01-18" @default.
- W269743404 modified "2023-09-27" @default.
- W269743404 title "Decomposition of hydrogen sulfide for small scale gas processing. Annual report, January 1992-December 1992" @default.
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