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• W2714154493 abstract "Sufficiently high oxygen ion conductivity of electrolyte is critical for good performance of low-temperature solid oxide fuel cells (LT-SOFCs). Notably, material conductivity, reliability, and manufacturing cost are the major barriers hindering LT-SOFC commercialization. Generally, surface properties control the physical and chemical functionalities of materials. Hereby, we report a Sm3+, Pr3+, and Nd3+ triple-doped ceria, exhibiting the highest ionic conductivity among reported doped-ceria oxides, 0.125 S cm-1 at 600 °C. It was designed using a two-step wet-chemical coprecipitation method to realize a desired doping for Sm3+ at the bulk and Pr3+/Nd3+ at surface domains (abbreviated as PNSDC). The redox couple Pr3+/Pr4+ contributes to the extraordinary ionic conductivity. Moreover, the mechanism for ionic conductivity enhancement is demonstrated. The above findings reveal that a joint bulk and surface doping methodology for ceria is a feasible approach to develop new oxide-ion conductors with high impacts on advanced LT-SOFCs." @default.
• W2714154493 created "2017-06-30" @default.
• W2714154493 creator A5042528673 @default.
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• W2714154493 date "2017-07-05" @default.
• W2714154493 modified "2023-10-03" @default.
• W2714154493 title "Superionic Conductivity of Sm³⁺, Pr³⁺, and Nd³⁺ Triple-Doped Ceria through Bulk and Surface Two-Step Doping Approach" @default.
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• W2714154493 doi "https://doi.org/10.1021/acsami.7b02224" @default.
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• W2714154493 hasPublicationYear "2017" @default.
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