Matches in SemOpenAlex for { <https://semopenalex.org/work/W2728657893> ?p ?o ?g. }
- W2728657893 endingPage "788" @default.
- W2728657893 startingPage "784" @default.
- W2728657893 abstract "The interfacial structure and dynamics of water in a microscopically confined geometry is imaged in three dimensions and on millisecond time scales. We developed a 3D wide-field second harmonic microscope that employs structured illumination. We image pH induced chemical changes on the curved and confined inner and outer surfaces of a cylindrical glass micro-capillary immersed in aqueous solution. The image contrast reports on the orientational order of interfacial water, induced by charge-dipole interactions between water molecules and surface charges. The images constitute surface potential maps. Spatially resolved surface pKa,s values are determined for the silica deprotonation reaction. Values range from 2.3<pKa,s<10.7, highlighting the importance of surface heterogeneities. Water molecules that rotate along an oscillating external electric field are also imaged. With this approach, real time movies of surface processes that involve flow, heterogeneities and potentials can be made, which will further developments in electrochemistry, geology, catalysis, biology, and microtechnology." @default.
- W2728657893 created "2017-07-14" @default.
- W2728657893 creator A5007873537 @default.
- W2728657893 creator A5025177026 @default.
- W2728657893 creator A5071525415 @default.
- W2728657893 creator A5075882864 @default.
- W2728657893 date "2017-08-25" @default.
- W2728657893 modified "2023-10-17" @default.
- W2728657893 title "Optical imaging of surface chemistry and dynamics in confinement" @default.
- W2728657893 cites W1504362703 @default.
- W2728657893 cites W1600870734 @default.
- W2728657893 cites W1985163522 @default.
- W2728657893 cites W1996353817 @default.
- W2728657893 cites W1999760255 @default.
- W2728657893 cites W2005124051 @default.
- W2728657893 cites W2007510454 @default.
- W2728657893 cites W2008315134 @default.
- W2728657893 cites W2013094701 @default.
- W2728657893 cites W2014965187 @default.
- W2728657893 cites W2017581879 @default.
- W2728657893 cites W2020556902 @default.
- W2728657893 cites W2032893627 @default.
- W2728657893 cites W2040040910 @default.
- W2728657893 cites W2042812633 @default.
- W2728657893 cites W2052250923 @default.
- W2728657893 cites W2058623136 @default.
- W2728657893 cites W2066153025 @default.
- W2728657893 cites W2067757940 @default.
- W2728657893 cites W2068808538 @default.
- W2728657893 cites W2074388484 @default.
- W2728657893 cites W2075495531 @default.
- W2728657893 cites W2076425962 @default.
- W2728657893 cites W2084597433 @default.
- W2728657893 cites W2087161209 @default.
- W2728657893 cites W2090272857 @default.
- W2728657893 cites W2093928990 @default.
- W2728657893 cites W2094806856 @default.
- W2728657893 cites W2096768639 @default.
- W2728657893 cites W2098681947 @default.
- W2728657893 cites W2100939380 @default.
- W2728657893 cites W2101192182 @default.
- W2728657893 cites W2104953138 @default.
- W2728657893 cites W2112596564 @default.
- W2728657893 cites W2117179092 @default.
- W2728657893 cites W2125271052 @default.
- W2728657893 cites W2128335842 @default.
- W2728657893 cites W2132480710 @default.
- W2728657893 cites W2145976479 @default.
- W2728657893 cites W2150377199 @default.
- W2728657893 cites W2152931265 @default.
- W2728657893 cites W2277760118 @default.
- W2728657893 cites W2282643467 @default.
- W2728657893 cites W2283357245 @default.
- W2728657893 cites W2302194893 @default.
- W2728657893 cites W2321117320 @default.
- W2728657893 cites W2323882202 @default.
- W2728657893 cites W2325601232 @default.
- W2728657893 cites W2328638068 @default.
- W2728657893 cites W2461688979 @default.
- W2728657893 cites W2511943864 @default.
- W2728657893 cites W2551673433 @default.
- W2728657893 cites W3022812332 @default.
- W2728657893 cites W3100359770 @default.
- W2728657893 cites W3104062667 @default.
- W2728657893 cites W4253606650 @default.
- W2728657893 doi "https://doi.org/10.1126/science.aal4346" @default.
- W2728657893 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/28729352" @default.
- W2728657893 hasPublicationYear "2017" @default.
- W2728657893 type Work @default.
- W2728657893 sameAs 2728657893 @default.
- W2728657893 citedByCount "84" @default.
- W2728657893 countsByYear W27286578932017 @default.
- W2728657893 countsByYear W27286578932018 @default.
- W2728657893 countsByYear W27286578932019 @default.
- W2728657893 countsByYear W27286578932020 @default.
- W2728657893 countsByYear W27286578932021 @default.
- W2728657893 countsByYear W27286578932022 @default.
- W2728657893 countsByYear W27286578932023 @default.
- W2728657893 crossrefType "journal-article" @default.
- W2728657893 hasAuthorship W2728657893A5007873537 @default.
- W2728657893 hasAuthorship W2728657893A5025177026 @default.
- W2728657893 hasAuthorship W2728657893A5071525415 @default.
- W2728657893 hasAuthorship W2728657893A5075882864 @default.
- W2728657893 hasBestOaLocation W27286578931 @default.
- W2728657893 hasConcept C113196181 @default.
- W2728657893 hasConcept C120665830 @default.
- W2728657893 hasConcept C121332964 @default.
- W2728657893 hasConcept C1276947 @default.
- W2728657893 hasConcept C147789679 @default.
- W2728657893 hasConcept C159467904 @default.
- W2728657893 hasConcept C171250308 @default.
- W2728657893 hasConcept C173523689 @default.
- W2728657893 hasConcept C178790620 @default.
- W2728657893 hasConcept C184651966 @default.
- W2728657893 hasConcept C185592680 @default.
- W2728657893 hasConcept C192562407 @default.
- W2728657893 hasConcept C2524010 @default.
- W2728657893 hasConcept C2776799497 @default.