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• W2729888082 abstract "Abstract By changing metal ions, three various transition metal coordination polymers based on different isopolymolybdates, [AgI(DTBA)(Mo2O6)] (1), [CuII3(DTBA)2(γ-Mo8O26)(H2O)6]·7H2O (2), and [CoII3(HDTBA)2(DTBA)2(γ-Mo8O26)(H2O)2]·6H2O (3) (HDTBA = 3,5-di(1,2,4-triazol-1-yl) benzoic acid) have been synthesized and characterized. In compounds 1–3, the ligand 3,5-di-[1,2,4]triazol-1-yl-benzoic acid (HDTBA) was in-situ transformed from the 3,5-di-[1,2,4]triazol-1-yl-benzonitrile (DTCN) under hydrothermal conditions and two kinds of isopolymolybdates formed, both of which were directly grafted by the in-situ ligand DTBA. When Ag+ ion was presented, a 3D framework 1 is constructed from {[Mo4O13](DTBA)2} building blocks. Replacing Ag+ with Cu2+ ion, compound 2 shows a (2,4,8)-connected framework based on {(γ-Mo8O26)(DTBA)2} building units. A {(γ-Mo8O26)(DTBA)2} building unit-based (4,4,8)-connected 3D framework 3 is obtained in the presence of Co2+ ions. The metal atoms may play key roles in tuning the various structures of compounds 1–3, as well as the different isopolymolybdates. The electrochemical properties and photocatalytic activities of compounds 1–3 have been investigated here." @default.
• W2729888082 created "2017-07-14" @default.
• W2729888082 creator A5029824045 @default.
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• W2729888082 date "2017-10-01" @default.
• W2729888082 modified "2023-09-27" @default.
• W2729888082 title "Metal ion-tuned coordination polymers based on different isopolymolybdates grafted by in-situ ligand" @default.
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• W2729888082 doi "https://doi.org/10.1016/j.poly.2017.06.033" @default.
• W2729888082 hasPublicationYear "2017" @default.
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