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• W2734489738 abstract "Sodium dodecylsulfate (SDS) - a simple single tailed surfactant (STS) can form stable vesicles from its micellar solution without any additives under the mediation of solid surfaces. To further understand the mechanism of this transition on the molecular level, molecular dynamics simulations are performed to study segments of SDS bilayers (as part of vesicles) in the bulk solution systematically, at the moment that the lower leaflet of bilayers already detached from solid surfaces. The SDS membrane would rather keep their bilayers structure than return to micelles when the initial interdigitated degree (δi) between alkyl chains is more than 8.0 ± 1.4%. And the interdigitated degree is always approaching to 31.7 ± 2.0% while the equilibrium is reached. The aggregates behave as curved bilayers, planar bilayers, perforated bilayers, and micelles with the increase of the lower leaflet cross-sectional area. Besides, the structures of salt bridge and water bridge structures are formed between DS− and Na+ ions or water molecules, which contribute to the stability of SDS bilayers. The distribution difference of the salt bridges along the direction of S-O axis between the two leaflets leads to the asymmetry of the bilayers, which plays supplementary role to the formation of bilayers curvature. We expect that this work help to shed light on the understanding of interface phenomena and the mechanism of simple single-tailed surfactant vesicle self-assembly on the molecular level." @default.
• W2734489738 created "2017-07-21" @default.
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• W2734489738 date "2017-11-01" @default.
• W2734489738 modified "2023-10-17" @default.
• W2734489738 title "Molecular dynamics simulation of sodium dodecylsulfate (SDS) bilayers" @default.
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• W2734489738 doi "https://doi.org/10.1016/j.jcis.2017.07.042" @default.
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