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- W2735698826 abstract "The study of novel metal-templated dynamic organocatalytic systems has led to the identification of CuSO4 as the most efficient template to assemble monofunctional prolinamide- and thiourea-modified pyridine ligands. The structural and electronic requirements to assemble an efficient catalyst have been disclosed: both pyridine ligands must bear a 1,3-substitution pattern, and the thiourea ligand serves as a reducing agent to copper(i) as well. Eventually, the cooperative effects achieved with such a simple system deliver high reaction rates and stereoselectivities at room temperature in the asymmetric aldol reaction, requiring only 1 mol% of copper salt." @default.
- W2735698826 created "2017-07-21" @default.
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- W2735698826 date "2017-01-01" @default.
- W2735698826 modified "2023-10-06" @default.
- W2735698826 title "A copper-templated, bifunctional organocatalyst: a strongly cooperative dynamic system for the aldol reaction" @default.
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- W2735698826 doi "https://doi.org/10.1039/c7ob01370a" @default.
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