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- W2737601331 abstract "The increasing number of experimental observations on highly concentrated electrolytes, such as self-assembly, multiple-time relaxation, and under-screening, emphasizes the paramount need for a formulation of a general framework that goes beyond the distinct modifications of the classical Poisson-Nernst-Planck equations. Using a standard free energy for electrolytes with phase separation properties and Onsager's energy dissipation methodology, new model equations for a ternary composition of solvent and ions are being derived. The model describes three distinct regions of interfacial and bulk structure. In particular, the model's predictions for screening length are in a qualitative agreement with the experimental results for both aqueous and organic solvents, and reveal a mechanism for the under-screening phenomenon." @default.
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- W2737601331 date "2017-07-21" @default.
- W2737601331 modified "2023-09-27" @default.
- W2737601331 title "From solvent free to dilute electrolytes: A unified continuum approach" @default.
- W2737601331 hasPublicationYear "2017" @default.
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