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- W2738536524 abstract "Abstract Highly efficient NaF-doped Li 4 SiO 4 sorbents were synthesized by sacrificial carbon template technology to overcome their typical kinetic limitations at low CO 2 concentrations. The samples were characterized by XRD, SEM, N 2 adsorption, XPS, differential scanning calorimetry (DSC), and thermogravimetric analyses (dynamic and isothermic). The results showed that co-doped sodium and fluorine were substituted for lithium and oxygen, respectively. Such doped features induced a high concentration of Li-O sites on the molten surface when absorbing CO 2 in a relatively wide temperature range (475–575 °C). This favorable characteristic greatly facilitated surface chemisorption processes, accelerated the transport of Li + and O 2− , and decreased the CO 2 diffusion resistance. Therefore, 3 wt.% NaF doping was used to reach a maximum absorption capacity (>33.0 wt.%) in a wide temperature range (475–575 °C) in 15 vol.% CO 2 . Moreover, the high capacity was maintained over 10 sorption/desorption cycles, suggesting that NaF-doped Li 4 SiO 4 sorbents have high potential for CO 2 capture." @default.
- W2738536524 created "2017-07-31" @default.
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- W2738536524 date "2017-10-01" @default.
- W2738536524 modified "2023-09-24" @default.
- W2738536524 title "Molten sodium-fluoride-promoted high-performance Li4SiO4-based CO2 sorbents at low CO2 concentrations" @default.
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- W2738536524 doi "https://doi.org/10.1016/j.apenergy.2017.07.072" @default.
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