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• W2739654865 endingPage "29450" @default.
• W2739654865 startingPage "29445" @default.
• W2739654865 abstract "Cu+-containing materials have drawn much attention in various applications because they are versatile, nontoxic, and low-cost. However, the difficulty of selective reduction and the poor stability of Cu+ species are now pretty much the agendas. Here, controlled construction of supported Cu+ sites in MIL-100(Fe) was realized under mild conditions (200 °C, 5 h) via a vapor-reduction strategy (VRS). Remarkably, the yield of Cu+ reaches 100%, which is quite higher than the traditional high-temperature autoreduction method with a yield less than 50% even at 700 °C for 12 h. More importantly, during the treatment via VRS some Fe3+ in MIL-100(Fe) are reduced to Fe2+, which prevent the frequently happened oxidation of Cu+ due to the higher oxidation potential of Fe2+. These properties make Cu+/MIL-100(Fe) efficient in the capture of typical aromatic sulfur, benzothiophene, with regard to both adsorption capacity and stability. To our knowledge, the stabilization of Cu+ using the oxidation tendency of supports is achieved for the first time, which may offer a new idea to utilize active sites with weak stability." @default.
• W2739654865 created "2017-08-08" @default.
• W2739654865 creator A5022863954 @default.
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• W2739654865 date "2017-07-27" @default.
• W2739654865 modified "2023-10-17" @default.
• W2739654865 title "Controlled Construction of Supported Cu⁺ Sites and Their Stabilization in MIL-100(Fe): Efficient Adsorbents for Benzothiophene Capture" @default.
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• W2739654865 doi "https://doi.org/10.1021/acsami.7b09300" @default.
• W2739654865 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/28745491" @default.
• W2739654865 hasPublicationYear "2017" @default.
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